@article{ISI:000468005400021,
title = {Freely Suspended, van der Waals Bound Organic Nanometer-Thin Functional
Films: Mechanical and Electronic Characterization},
author = {Lilian S Schaffroth and Jakob Lenz and Veit Giegold and Maximilian Koegl and Achim Hartschuh and Thomas R Weitz},
doi = {10.1002/adma.201808309},
issn = {0935-9648},
year = {2019},
date = {2019-04-01},
journal = {ADVANCED MATERIALS},
volume = {31},
number = {16},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000466053300004,
title = {Scaffold-Induced Diketopyrrolopyrrole Molecular Stacks in a Covalent
Organic Framework},
author = {Sabrina Rager and Andreas C Jakowetz and Bappaditya Gole and Florian Beuerle and Dana D Medina and Thomas Bein},
doi = {10.1021/acs.chemmater.8b02882},
issn = {0897-4756},
year = {2019},
date = {2019-04-01},
journal = {CHEMISTRY OF MATERIALS},
volume = {31},
number = {8},
pages = {2707-2712},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Wild, Stefan ; Fickert, Michael ; Mitrovic, Aleksandra ; Lloret, Vicent ; Neiss, Christian ; Vidal-Moya, José Alejandro ; Rivero-Crespo, Miguel Ángel ; Leyva-Pérez, Antonio ; Werbach, Katharina ; Peterlik, Herwig ; Grabau, Mathias ; Wittkämper, Haiko ; Papp, Christian ; Steinrück, Hans-Peter ; Pichler, Thomas ; Görling, Andreas ; Hauke, Frank ; Abellán, Gonzalo ; Hirsch, Andreas
@article{Wild2019,
title = {Lattice Opening upon Bulk Reductive Covalent Functionalization of Black Phosphorus},
author = {Wild, Stefan and Fickert, Michael and Mitrovic, Aleksandra and Lloret, Vicent and Neiss, Christian and Vidal-Moya, José Alejandro and Rivero-Crespo, Miguel Ángel and Leyva-Pérez, Antonio and Werbach, Katharina and Peterlik, Herwig and Grabau, Mathias and Wittkämper, Haiko and Papp, Christian and Steinrück, Hans-Peter and Pichler, Thomas and Görling, Andreas and Hauke, Frank and Abellán, Gonzalo and Hirsch, Andreas},
doi = {10.1002/anie.201811181},
year = {2019},
date = {2019-03-21},
journal = {Angewandte Chemie International Edition},
volume = {58},
number = {17},
pages = {5763-5768},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
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title = {Intricacies of DFT plus U, Not Only in a Numeric Atom Centered Orbital
Framework},
author = {Matthias Kick and Karsten Reuter and Harald Oberhofer},
doi = {10.1021/acs.jctc.8b01211},
issn = {1549-9618},
year = {2019},
date = {2019-03-01},
journal = {JOURNAL OF CHEMICAL THEORY AND COMPUTATION},
volume = {15},
number = {3},
pages = {1705-1718},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000462624900017,
title = {Dielectric-Semiconductor Interface Limits Charge Carrier Motion at Elevated Temperatures and Large Carrier Densities in a High-Mobility Organic Semiconductor},
author = {Ilja Vladimirov and Sebastian Mueller and Roelf-Peter Baumann and Thomas Gesser and Zahra Molla and Souren Grigorian and Anna Koehler and Heinz Baessler and Ullrich Pietsch and Ralf Thomas Weitz},
doi = {10.1002/adfm.201807867},
issn = {1616-301X},
year = {2019},
date = {2019-03-01},
journal = {ADVANCED FUNCTIONAL MATERIALS},
volume = {29},
number = {12},
pages = {1807867},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000462260000061,
title = {Morphology Tuning of ZnO/P3HT/P3HT-b-PEO Hybrid Films Deposited via
Spray or Spin Coating},
author = {Kun Wang and Nuri Hohn and Lucas P Kreuzer and Tobias Widmann and Martin Haese and Jean-Francois Moulin and Peter Mueller-Buschbaum},
doi = {10.1021/acsami.9b00599},
issn = {1944-8244},
year = {2019},
date = {2019-03-01},
journal = {ACS APPLIED MATERIALS & INTERFACES},
volume = {11},
number = {11},
pages = {10998-11005},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000462661900019,
title = {A top-down strategy identifying molecular phase stabilizers to overcome
microstructure instabilities in organic solar cells},
author = {Chaohong Zhang and Thomas Heumueller and Salvador Leon and Wolfgang Gruber and Klaus Burlafinger and Xiaofeng Tang and Jose D Perea and Isabell Wabra and Andreas Hirsch and Tobias Unruh and Ning Li and Christoph J Brabec},
doi = {10.1039/c8ee03780a},
issn = {1754-5692},
year = {2019},
date = {2019-03-01},
journal = {ENERGY & ENVIRONMENTAL SCIENCE},
volume = {12},
number = {3},
pages = {1078-1087},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000463234600016,
title = {Preparation and Characterization of a pi-Conjugated Donor-Acceptor
System Containing the Strongly Electron-Accepting Tetraphenylborolyl
Unit},
author = {Michael Meier and Lei Ji and Joern Nitsch and Ivo Krummenacher and Andrea Deissenberger and Dominic Auerhammer and Marius Schaefer and Todd B Marder and Holger Braunschweig},
doi = {10.1002/chem.201805454},
issn = {0947-6539},
year = {2019},
date = {2019-03-01},
journal = {CHEMISTRY-A EUROPEAN JOURNAL},
volume = {25},
number = {18},
pages = {4707-4712},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{Schlipf2019,
title = {Shedding Light on the Moisture Stability of 3D/2D Hybrid Perovskite Heterojunction Thin Films},
author = {Schlipf, Johannes and Hu, Yinghong and Pratap, Shambhavi and Bießmann, Lorenz and Hohn, Nuri and Porcar, Lionel and Bein, Thomas and Docampo, Pablo and Müller-Buschbaum, Peter},
doi = {10.1021/acsaem.9b00005},
year = {2019},
date = {2019-02-06},
journal = {ACS Applied Energy Materials},
volume = {2},
number = {2},
pages = {1011-1018},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000459504400005,
title = {Emergence of lead halide perovskite colloidal dispersions through
aggregation and fragmentation: insights from the nanoscale to the
mesoscale},
author = {Shambhavi Pratap and Elisabeth Keller and Peter Mueller-Buschbaum},
doi = {10.1039/c8nr09853k},
issn = {2040-3364},
year = {2019},
date = {2019-02-01},
journal = {NANOSCALE},
volume = {11},
number = {8},
pages = {3495-3499},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
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title = {Multifunctional and Tunable Surfaces Based on Pyrene Functionalized
Nanoparticles},
author = {Judith E Wittmann and Lisa M S Stiegler and Christian Henkel and Johannes Traeg and Klaus Goetz and Tobias Unruh and Dirk Zahn and Andreas Hirsch and Dirk Guldi and Marcus Halik},
doi = {10.1002/admi.201801930},
issn = {2196-7350},
year = {2019},
date = {2019-02-01},
journal = {ADVANCED MATERIALS INTERFACES},
volume = {6},
number = {4, SI},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000459323700025,
title = {A Self-Assembled Unit Comprising 12 Squaraine Dyes Built Up from Two
Star-Shaped Hexasquarainyl-Benzene Molecules},
author = {Maximilian H Schreck and Merle I S Roehr and Timothy Clark and Vladimir Stepanenko and Frank Wuerthner and Christoph Lambert},
doi = {10.1002/chem.201805685},
issn = {0947-6539},
year = {2019},
date = {2019-02-01},
journal = {CHEMISTRY-A EUROPEAN JOURNAL},
volume = {25},
number = {11},
pages = {2831-2839},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Kynaston, Emily L; Winchell, K J; Yee, Patrick Y; Manion, Joseph G; Hendsbee, Arthur D; Li, Yuning; Huettner, Sven; Tolbert, Sarah H; Seferos, Dwight S
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title = {Poly(3-alkylthiophene)-block-poly(3-alkylselenophene)s: Conjugated
Diblock Co-polymers with Atypical Self-Assembly Behavior},
author = {Emily L Kynaston and K J Winchell and Patrick Y Yee and Joseph G Manion and Arthur D Hendsbee and Yuning Li and Sven Huettner and Sarah H Tolbert and Dwight S Seferos},
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issn = {1944-8244},
year = {2019},
date = {2019-02-01},
journal = {ACS APPLIED MATERIALS & INTERFACES},
volume = {11},
number = {7},
pages = {7174-7183},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000459223200018,
title = {Reduction of the Fluorescence Transition Dipole Moment by Excitation
Localization in a Vibronically Coupled Squaraine Dimer},
author = {Henning Marciniak and Nina Auerhammer and Sophie Ricker and Alexander Schmiedel and Marco Holzapfel and Christoph Lambert},
doi = {10.1021/acs.jpcc.8b11957},
issn = {1932-7447},
year = {2019},
date = {2019-02-01},
journal = {JOURNAL OF PHYSICAL CHEMISTRY C},
volume = {123},
number = {6},
pages = {3426-3432},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000458937800039,
title = {Finding the Right Bricks for Molecular Legos: A Data Mining Approach to
Organic Semiconductor Design},
author = {Christian Kunkel and Christoph Schober and Johannes T Margraf and Karsten Reuter and Harald Oberhofer},
doi = {10.1021/acs.chemmater.8b04436},
issn = {0897-4756},
year = {2019},
date = {2019-02-01},
journal = {CHEMISTRY OF MATERIALS},
volume = {31},
number = {3},
pages = {969-978},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000459642800001,
title = {Quantifying Figures of Merit for Localized Surface Plasmon Resonance
Applications: A Materials Survey},
author = {Brock Doiron and Monica Mota and Matthew P Wells and Ryan Bower and Andrei Mihai and Yi Li and Lesley F Cohen and Neil McN. Alford and Peter K Petrov and Rupert F Oulton and Stefan A Maier},
doi = {10.1021/acsphotonics.8b01369},
issn = {2330-4022},
year = {2019},
date = {2019-02-01},
journal = {ACS PHOTONICS},
volume = {6},
number = {2},
pages = {240-259},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000459910900054,
title = {Amphiphilic diblock copolymer-mediated structure control in nanoporous
germanium-based thin films},
author = {Nuri Hohn and Andreas E Hetzenecker and Michael A Giebel and Sebastian Geier and Lorenz Biessmann and Volker Koerstgens and Nitin Saxena and Johannes Schlipf and Wiebke Ohm and Peter S Deimel and Francesco Allegretti and Johannes V Barth and Stephan V Roth and Thomas F Faessler and Peter Mueller-Buschbaum},
doi = {10.1039/c8nr09427f},
issn = {2040-3364},
year = {2019},
date = {2019-01-01},
journal = {NANOSCALE},
volume = {11},
number = {4},
pages = {2048-2055},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000457414600016,
title = {Generalized molecular solvation in non-aqueous solutions by a single
parameter implicit solvation scheme},
author = {Christoph Hille and Stefan Ringe and Martin Deimel and Christian Kunkel and William E Acree and Karsten Reuter and Harald Oberhofer},
doi = {10.1063/1.5050938},
issn = {0021-9606},
year = {2019},
date = {2019-01-01},
journal = {JOURNAL OF CHEMICAL PHYSICS},
volume = {150},
number = {4},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000457067500008,
title = {Singlet Fission in Combinatorial Diketopyrrolopyrrole-Rylene
Supramolecular Films},
author = {Andrew M Levine and Christoph Schierl and Bettina S Basel and Mehroz Ahmed and Braden A Camargo and Dirk M Guldi and Adam B Braunschweig},
doi = {10.1021/acs.jpcc.8b09593},
issn = {1932-7447},
year = {2019},
date = {2019-01-01},
journal = {JOURNAL OF PHYSICAL CHEMISTRY C},
volume = {123},
number = {3},
pages = {1587-1595},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000460162900065,
title = {Nanographene favors electronic interactions with an electron acceptor
rather than an electron donor in a planar fused push-pull conjugate},
author = {Michel Volland and Ping Zhou and Leonie Wibmer and Robert Haener and Silvio Decurtins and Shi-Xia Liu and Dirk M Guldi},
doi = {10.1039/c8nr06961a},
issn = {2040-3364},
year = {2019},
date = {2019-01-01},
journal = {NANOSCALE},
volume = {11},
number = {3},
pages = {1437-1441},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000457575300001,
title = {Intermolecular Singlet Fission in Unsymmetrical Derivatives of Pentacene
in Solution},
author = {Ruben Casillas and Matthias Adam and Pedro B Coto and Andreas R Waterloo and Johannes Zirzlmeier and Seelam Rajagopala Reddy and Frank Hampel and Robert McDonald and Rik R Tykwinski and Michael Thoss and Dirk M Guldi},
doi = {10.1002/aenm.201802221},
issn = {1614-6832},
year = {2019},
date = {2019-01-01},
journal = {ADVANCED ENERGY MATERIALS},
volume = {9},
number = {2},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000455111100021,
title = {Ionic-Liquid Doping Enables High Transconductance, Fast Response Time,
and High Ion Sensitivity in Organic Electrochemical Transistors},
author = {Xihu Wu and Abhijith Surendran and Jieun Ko and Oliver Filonik and Eva M Herzig and Peter Mueller-Buschbaum and Wei Lin Leong},
doi = {10.1002/adma.201805544},
issn = {0935-9648},
year = {2019},
date = {2019-01-01},
journal = {ADVANCED MATERIALS},
volume = {31},
number = {2},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000453601400007,
title = {Dithienobenzimidazole-containing conjugated donor-acceptor polymers:
Synthesis and characterization},
author = {Jared D Harris and Markus Stihl and Hans-Werner Schmidt and Kenneth R Carter},
doi = {10.1002/pola.29284},
issn = {0887-624X},
year = {2019},
date = {2019-01-01},
journal = {JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY},
volume = {57},
number = {1},
pages = {60-69},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000457067300065,
title = {Composition Morphology Correlation in PTB7-Th/PC71 BM Blend Films for
Organic Solar Cells},
author = {Lin Song and Weijia Wang and Edoardo Barabino and Dan Yang and Volker Koerstgens and Peng Zhang and Stephan V Roth and Peter Mueller-Buschbaum},
doi = {10.1021/acsami.8b20316},
issn = {1944-8244},
year = {2019},
date = {2019-01-01},
journal = {ACS APPLIED MATERIALS & INTERFACES},
volume = {11},
number = {3},
pages = {3125-3135},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000456422500005,
title = {Why Tin-Doping Enhances the Efficiency of Hematite Photoanodes for Water Splitting-The Full Picture},
author = {Alexander G Hufnagel and Hamidreza Hajiyani and Siyuan Zhang and Tong Li and Olga Kasian and Baptiste Gault and Benjamin Breitbach and Thomas Bein and Dina Fattakhova-Rohlfing and Christina Scheu and Rossitza Pentcheva},
doi = {10.1002/adfm.201804472},
issn = {1616-301X},
year = {2018},
date = {2018-12-01},
journal = {ADVANCED FUNCTIONAL MATERIALS},
volume = {28},
number = {52},
pages = {1804472},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000454567200006,
title = {Capping nido-Nonagermanide Clusters with M-PPh3 and Dynamics in
Solution: Synthesis and Structure of closo-[(Me3Si)(3)Si](3)Et[Ge9M](PPh3) (M = Ni, Pt)},
author = {Sabine Frischhut and Felix Kaiser and Wilhelm Klein and Markus Drees and Fritz E Kuehn and Thomas F Faessler},
doi = {10.1021/acs.organomet.8b00459},
issn = {0276-7333},
year = {2018},
date = {2018-12-01},
journal = {ORGANOMETALLICS},
volume = {37},
number = {24},
pages = {4560-4567},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000452490800028,
title = {Synergy of light harvesting and energy transfer as well as short-range
charge shift reactions in multicomponent conjugates},
author = {Ettore Fazio and Kim A Winterfeld and Ana Lopez-Perez and Tomas Torres and Dirk M Guldi and Gema de la Torre},
doi = {10.1039/c8nr08438f},
issn = {2040-3364},
year = {2018},
date = {2018-12-01},
journal = {NANOSCALE},
volume = {10},
number = {47},
pages = {22400-22408},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000454383400043,
title = {Selective Photocatalytic C-F Borylation of Polyfluoroarenes by Rh/Ni
Dual Catalysis Providing Valuable Fluorinated Arylboronate Esters},
author = {Ya-Ming Tian and Xiao-Ning Guo and Maximilian W Kuntze-Fechner and Ivo Krummenacher and Holger Braunschweig and Udo Radius and Andreas Steffen and Todd B Marder},
doi = {10.1021/jacs.8b09790},
issn = {0002-7863},
year = {2018},
date = {2018-12-01},
journal = {JOURNAL OF THE AMERICAN CHEMICAL SOCIETY},
volume = {140},
number = {50},
pages = {17612-17623},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000454216900007,
title = {X-ray study of anisotropically shaped metal halide perovskite nanoparticles in tubular pores},
author = {Janina Melanie Roemer and Stepan Demchyshyn and Anton Boehm and Olof Gutowski and Kilian Frank and Niyazi Serdar Sariciftci and Martin Kaltenbrunner and Bert Nickel},
doi = {10.1063/1.5054271},
issn = {0003-6951},
year = {2018},
date = {2018-12-01},
journal = {APPLIED PHYSICS LETTERS},
volume = {113},
number = {25},
pages = {251901},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000453441300003,
title = {Overcoming efficiency and stability limits in water-processing
nanoparticular organic photovoltaics by minimizing microstructure
defects},
author = {Chen Xie and Thomas Heumueller and Wolfgang Gruber and Xiaofeng Tang and Andrej Classen and Isabel Schuldes and Matthew Bidwell and Andreas Spaeth and Rainer H Fink and Tobias Unruh and Iain McCulloch and Ning Li and Christoph J Brabec},
doi = {10.1038/s41467-018-07807-5},
issn = {2041-1723},
year = {2018},
date = {2018-12-01},
journal = {NATURE COMMUNICATIONS},
volume = {9},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000452693800026,
title = {Enforcing Extended Porphyrin J-Aggregate Stacking in Covalent Organic
Frameworks},
author = {Niklas Keller and Mona Calik and Dmitry Sharapa and Himadri R Soni and Peter M Zehetmaier and Sabrina Rager and Florian Auras and Andreas C Jakowetz and Andreas Goerling and Timothy Clark and Thomas Bein},
doi = {10.1021/jacs.8b08086},
issn = {0002-7863},
year = {2018},
date = {2018-12-01},
journal = {JOURNAL OF THE AMERICAN CHEMICAL SOCIETY},
volume = {140},
number = {48},
pages = {16544-16552},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000452235600024,
title = {Chemical Cutting of Perovskite Nanowires into Single-Photon Emissive Low-Aspect-Ratio CsPbX3 (X = Cl, Br, I) Nanorods},
author = {Yu Tong and Ming Fu and Eva Bladt and He Huang and Alexander F Richter and Kun Wang and Peter Mueller-Buschbaum and Sara Bals and Philippe Tamarat and Brahim Lounis and Jochen Feldmann and Lakshminarayana Polavarapu},
doi = {10.1002/anie.201810110},
issn = {1433-7851},
year = {2018},
date = {2018-12-01},
journal = {ANGEWANDTE CHEMIE-INTERNATIONAL EDITION},
volume = {57},
number = {49},
pages = {16094-16098},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000452650200013,
title = {Fine-tuning of the chemical structure of photoactive materials for
highly efficient organic photovoltaics},
author = {Baobing Fan and Xiaoyan Du and Feng Liu and Wenkai Zhong and Lei Ying and Ruihao Xie and Xiaofeng Tang and Kang An and Jingming Xin and Ning Li and Wei Ma and Christoph J Brabec and Fei Huang and Yong Cao},
doi = {10.1038/s41560-018-0263-4},
issn = {2058-7546},
year = {2018},
date = {2018-12-01},
journal = {NATURE ENERGY},
volume = {3},
number = {12},
pages = {1051-1058},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000450456900001,
title = {A Feynman dispersion correction: a proof of principle for MNDO},
author = {Maximilian Kriebel and Konstantin Weber and Timothy Clark},
doi = {10.1007/s00894-018-3874-6},
issn = {1610-2940},
year = {2018},
date = {2018-12-01},
journal = {JOURNAL OF MOLECULAR MODELING},
volume = {24},
number = {12},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{ISI:000449708500085,
title = {New synthesized ionic liquid functionalized graphene oxide: Synthesis,
characterization and its nanocomposite with conjugated polymer as
effective electrode materials in an energy storage device},
author = {Farshad Boorboor Ajdari and Elaheh Kowsari and Ali Ehsani and Milan Schorowski and Tayebeh Ameri},
doi = {10.1016/j.electacta.2018.09.177},
issn = {0013-4686},
year = {2018},
date = {2018-12-01},
journal = {ELECTROCHIMICA ACTA},
volume = {292},
pages = {789-804},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
@article{Song_2018,
title = {Understanding macroscale functionality of metal halide perovskites in terms of nanoscale heterogeneities},
author = {Tze-Bin Song and Ian D Sharp and Carolin M Sutter-Fella},
doi = {10.1088/2515-7655/aaeee5},
year = {2018},
date = {2018-12-01},
journal = {Journal of Physics: Energy},
volume = {1},
number = {1},
pages = {011002},
publisher = {IOP Publishing},
abstract = {Hybrid metal halide perovskites have shown an unprecedented rise as semiconductor building blocks for solar energy conversion and light-emitting applications. Currently, the field moves empirically towards more and more complex chemical compositions, including mixed halide quadruple cation compounds that allow optical properties to be tuned and show promise for better stability. Despite tremendous progress in the field, there is a need for better understanding of mechanisms of efficiency loss and instabilities to facilitate rational optimization of composition. Starting from the device level and then diving into nanoscale properties, we highlight how structural and compositional heterogeneities affect macroscopic optoelectronic characteristics. Furthermore, we provide an overview of some of the advanced spectroscopy and imaging methods that are used to probe disorder and non-uniformities. A unique feature of hybrid halide perovskite compounds is the propensity for these heterogeneities to evolve in space and time under relatively mild illumination and applied electric fields, such as those found within active devices. This introduces an additional challenge for characterization and calls for application of complimentary probes that can aid in correlating the properties of local disorder with macroscopic function, with the ultimate goal of rationally tailoring synthesis towards optimal structures and compositions.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Hybrid metal halide perovskites have shown an unprecedented rise as semiconductor building blocks for solar energy conversion and light-emitting applications. Currently, the field moves empirically towards more and more complex chemical compositions, including mixed halide quadruple cation compounds that allow optical properties to be tuned and show promise for better stability. Despite tremendous progress in the field, there is a need for better understanding of mechanisms of efficiency loss and instabilities to facilitate rational optimization of composition. Starting from the device level and then diving into nanoscale properties, we highlight how structural and compositional heterogeneities affect macroscopic optoelectronic characteristics. Furthermore, we provide an overview of some of the advanced spectroscopy and imaging methods that are used to probe disorder and non-uniformities. A unique feature of hybrid halide perovskite compounds is the propensity for these heterogeneities to evolve in space and time under relatively mild illumination and applied electric fields, such as those found within active devices. This introduces an additional challenge for characterization and calls for application of complimentary probes that can aid in correlating the properties of local disorder with macroscopic function, with the ultimate goal of rationally tailoring synthesis towards optimal structures and compositions.
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